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Publications

Actinide Facility

Journal Articles

  1. Neptunium Redox Speciation, M. R. Antonio, C. W. Williams,
    J.-P. Blaudeau and B. E. Bursten, Radiochimica Acta, 89 (1),
    17-25 (2001).
  2. The Coordination Geometry of Np(VII) in Alkaline Solution,
    C. W. Williams, J.-P. Blaudeau, J. C. Sullivan, M. R. Antonio, B. E.
    Bursten, and L. Soderholm, J. Amer. Chem. Soc. 123 (2001) 4346-4347.
  3. The Formation and Stability of [EuP5W30O110]12- and
    [AmP5W30O110]12-, C. W. Williams, M. R. Antonio and L. Soderholm,
    J. Alloys Cmpds. 303-304 (2000) 509-513.
  4. The Influence of Desulfovibrio Desulfuricans on Neptunium Chemistry,
    L. Soderholm, C.W. Williams, M. R. Antonio, M. L. Tischler, and
    M. Markos, Mater. Res. Soc. Symp. Proc. (2000) 590 (Applications
    of Synchrotron Radiation Techniques to Materials Science V), 27-32.
  5. Studies of Local Structures of Cm3+ in Borosilicate Glass using Laser
    and X-Ray Spectroscopic Methods and Computational Modeling,
    G. K. Liu, V. V. Zhorin, M. R. Antonio, S. T. Li, C. W. Williams and
    L. Soderholm, J. Chem. Phys. 112, 1489-1496 (2000)
  6. The Magnetic Properties of Pr in the High-Tc Superconductor
    Pb2Sr2R1-xCaxCu3O8: (x=0 and 0.5), U. Staub, L. Soderholm,
    S. Skanthakumar, R. Osborn, F. Fauth and C. Ritter, Physica C
    333, 13-22 (2000)
  7. Valence Determination as a Function of Doping in SrBa2Cu3O7,
    U. Staub, L. Soderholm, S. R. Wasserman, F. Fauth, A. G. O. Conner,
    M. J. Kramer, B. Patterson, M. Shi and M. Knapp, Phys. Rev. B
    61, 1548-1554 (2000)
  8. Redox Behaviour of Cerium in Heteropolyoxotungstate Complexes,
    M. R. Antonio, L. Soderholm, C. W. Williams, N. Ullah and
    L. Francesconi, J. Chem. Soc., Dalton Trans., 1999, 3825-3830 (1999)
  9. X-Ray Resonant Exchange Scattering from Transuranium Compounds,
    D. Mannix, S. Langridge, G. H. Lander, J. Rebizant, M. J. Longfield,
    W. G. Stirling, W. J. Nuttall, S. Coburn, S. Wasserman and
    L. Soderholm, Physica B 262, 125-140 (1999)
  10. XANES Spectroelectrochemistry:  A New Tool for Determining
    Formal Potentials, L. Soderholm, M. R. Antonio, C. W. Williams
    and S. R. Wasserman, Anal. Chem. 71, 4622-4628 (1999)
  11. Structure and Magnetic Properties of the High Tc Related Phase
    Cm2CuO4, L. Soderholm, S. Skanthakumar and C. W. Williams,
    Phys. Rev. B 60, 4302-4308 (1999-II)
  12. X-Ray Excited Optical Luminescence (XEOL) Detection of X-Ray
    Absorption Fine Structure (XAFS), L. Soderholm, G. K. Liu,
    M. R. Antonio and F. W. Lytle, J. Chem. Phys. 109, 6745-6752 (1998)
  13. The Effects of Surface Modification on the Interlayer Chemistry of
    Iron in a Smectite Clay, S. Wasserman, L. Soderholm and U. Staub,
    Chem. of Materials 10, 559-566 (1998)
  14. Surface Contamination of Single Crystal PuSb, S. R. Wasserman,
    L. Soderholm, J. Rebizant and G. H. Lander, J. Alloys and
    Compounds 271/273, 882-886 (1998)
  15. Tetravalent Uranium in Calcite, N. C. Sturchio, M. R. Antonio,
    L. Soderholm, S. R. Sutton and J. C. Brannon, Science 281,
    971-973 (1998)
  16. Synthesis and Characterization of Actinide-Exchanged Preyssler
    Heteropolyanions [AnP5W30O110]n-, An=Th, Am, Cm,
    M. R. Antonio, C. W. Williams and L. Soderholm, J. Alloys and
    Compounds 271/273, 846-849 (1998)
  17. Coordination and Valence of Europium in [Eu(alpha-2- s2W17O61)2]17-
    and [Eu(W5O18)2]9-, M. R. Antonio, L. Soderholm, G. Jennings,
    L. C. Francesconi, M. Dankova and J. Bartis, J. Alloys and
    Compounds 275/277, 827-830 (1998)
  18. The Structure of Uranium in Surface Modified Clays, D. M. Giaquinta,
    S. E. Yuchs, L. Soderholm and S. R. Wasserman, J. Alloys and
    Compounds 249, 142-145 (1997)
  19. In Situ X-Ray Absorption Fine Structure and Optical Reflectance
    Studies of Electrodisposited Nickel Hydrous Oxide Films in
    Alkaline Electrolytes, Y. Hu, I. T. Bae, Y. Mo, M. R. Antonio
    and D. A. Scherson, Can. J. Chem. 75, 1721-1729 (1997)
  20. In Situ X-Ray Absorption Fine Structure Studies of a Manganese
    Dioxide Electrode in a Rechargeable MnO2/Zn Alkaline Battery
    Environment, Y. Mo, Y. Hu, I. T. Bae, B. Miller, M. R. Antonio
    and D. A. Scherson, J. Electrochem. Soc. 144, 1598-1603 (1997)
  21. In Situ Fe K-Edge X-Ray Absorption Fine Structure of a Pyrite
    Electrode in an Li/Polyethylene Oxide (LiClO4/FeS2) Battery
    Environment, D. A. Totir, I. T. Bae, Y. Hu, M. R. Antonio,
    M. A. Stan and D. A. Scherson, J. Phys. Chem. B 101,
    9751-9756 (1997)
  22. EXAFS Studies of Cesium Complexation by Dibenzo-Crown
    Ethers in Tri-n-butyl Phosphate, M. R. Antonio, M. L. Dietz,
    M. P. Jensen, L. Soderholm and E. P. Horwitz, Inorg. Chim.
    Acta 255, 13-20 (1997)
  23. Design of Spectroelectrochemical Cell for In Situ X-Ray
    Absorption Fine Structure Measurements of Bulk Solution
    Species, M. R. Antonio, L. Soderholm and I. Song, J. Appl.
    Electrochem. 27, 784-792 (1997)
  24. The Wave Vector Dependence of Intermultiplet Transitions
    in EuBa2Cu3Ox (x=6.1 and 7):  An Inelastic Neutron Scattering
    Study, U. Staub, R. Osborn, E. Balcar, L. Soderholm and
    V. Trounov, Phys. Rev. B 55, 11629-11626 (1997)
  25. Local Environments of Erbium and Lutetium in Sodium Silicate
    Glasses, M. R. Antonio, L. Soderholm and A. J. G. Ellison,
    J. Alloys and Compounds 250, 536-540 (1997)
  26. Implications of the Unusual Redox Behaviour Exhibited by the
    Heteropolyanion [EuP5W30O110]12-, M. R. Antonio and
    L. Soderholm, J. Alloys and Compounds 250, 541-543 (1997)
  27. Nanoscale Encapsulation:  The Structure of Cations in Hydrophobic
    Microporous Aluminosilicates, S. R. Wasserman, S. E. Yuchs,
    D. Giaquinta, L. Soderholm and K. Song, J. Phys. IV 7,
    803-807 (1997)
  28. Oxidation State of the Unusual Rare Earth (R = Ce, Pr and Tb) in
    Double-layer High-Tc Superconductors, U. Staub, L. Soderholm,
    S. Skanthakumar and M. R. Antonio, J. Phys. IV 7, 1077-1079
    (1997)
  29. Importance of the Magnetic Ground State of Pr for Tc Suppression
    in High-Tc Superconductors, U. Staub, L. Soderholm,
    S. Skanthakumar, R. Osborn and F. Fauth, Europhys. Lett.
    39, 663-668 (1997)
  30. Uranium Speciation in Glass Corrosion Layers: An XAFS Study,
    B. M. Biwer, L. Soderholm, R. G. Greegor and F. W. Lytle,
    Mat. Res. Soc. Symp. Proc. 465, 229-236 (1997)
  31. The Effects of Surface Modification on the Speciation of Metal
    Ions Intercalated into Aluminosilicates, S. R. Wasserman,
    D. M. Giaquinta, S. E. Yuchs and L. Soderholm, Mat. Res.
    Soc. Symp. Proc. 465, 473-480 (1997)
  32. The Speciation of Uranium in a Smectite Clay: Evidence for
    Catalysed Uranyl Reduction, D. M. Giaquinta, L. Soderholm,
    S. E. Yuchs and S. R. Wasserman, Radiochim. Acta 76(3),
    113-121 (1997)
  33. Quasi Two-dimensional Magnetic Order of Tb3+ Spins in
    Pb2Sr2Tb1-xCaxCu3O8 (x=0 and 0.5), U. Staub, L. Soderholm,
    S. Skanthakumar, S. Rosenkranz, C. Ritter and W. Kagunya,
    Z. Phys. B 104, 37-43 (1997)
  34. The Effect of f-ion Valence on Superconductivity in the Series
    Pb2Sr2RCu3O8 (R=Ce, Pr, Tb, and Am) , L. Soderholm,
    S. Skanthakumar, U. Staub, M. R. Antonio and C. W. Williams,
    J. Alloys and Compounds 250, 623-626 (1997)
  35. Magnetic Properties of Series Pb2Sr2PrCu3O8, U. Staub,
    S. Skanthakumar, L. Soderholm and R. Osborn, J. Alloys
    and Compounds 250, 581-584 (1997)
  36. Tb Spin Correlations in Pb2Sr2Tb0.5Ca0.5Cu3O8, U. Staub,
    L. Soderholm, S. Skanthakumar, S. Rosenkranz, C. Ritter
    and W. Kagunja, Europhys. Lett. 34, 447 (1996)
  37. The Synthesis and Magnetic Properties of the Superconductor-
    Related Series Pb2Sr2AmCu3O8, L. Soderholm, C. Williams,
    S. Skanthakumar, M. R. Antonio and S. Conradson, Z. Phys. B
    101, 539 (1996)
  38. Oxidation State of Ce in Pb2Sr2Ce1-xCaxCu3O8,
    S. Skanthakumar and L. Soderholm, Phys. Rev. B 53, 920 (1996)
  39. The Magnetic Properties of R in Pb2Sr2(R/Ca)Cu3O8 (R=Ho
    and Er), L. Soderholm, C.-K. Loong, U. Staub, S. Skanthakumar,
    J. Simon Xue, J. P. Hammonds, J. E. Greedan and M. Marc,
    Physica C 246, 11 (1995)
  40. Oxidation State and Magnetic Properties of Pb2Sr2Tb1-xYxCu3O8,
    U. Staub, L. Soderholm, S. Skanthakumar and M. R. Antonio,
    Phys. Rev. B 52, 9736 (1995)
  41. The Oxidation State and Magnetic Behavior of Tb in High-Tc
    Related Materials, L. Soderholm, U. Staub, S. Skanthakumar and
    M. R. Antonio, Mat. Res. Soc. Symp. Proc. 376, 529 (1995)
  42. Quadrupolar Effects on the Temperature Dependence of the
    Lattice Parameters in HoP1-xVxO4, S. Skanthakumar,
    C.-K. Loong, L. Soderholm, J. W. Richardson, Jr.,
    M. M. Abraham and L. A. Boatner, Phys. Rev. B
    51, 5644 (1995)
  43. Crystal-Field Excitations and Magnetic Properties of Ho3+
    in HoVO4, S. Skanthakumar, C.-K. Loong, L. Soderholm,
    M. M. Abraham and L. A. Boatner, Phys. Rev. B 51,
    12451 (1995)
  44. Anomalous Temperature Dependence of the Lattice
    Parameters in HoPO4 and HoVO4:  Rare-Earth
    Quadrupolar Effects, S. Skanthakumar, C.-K. Loong,
    L. Soderholm, J. W. Richardson, Jr., J. Nipko, M. M. Abraham
    and L. A. Boatner, J. Alloys and Compounds 225, 595 (1995)

IN PRESS

  1. Synchrotron X-Radiation Study of Illitic Clays from the Cigar Lake
    Uranium Deposit, Northern Saskatchewan, J. Percival, S. Skanthakumar,
    L. Soderholm, P.C. Burns and A. Locock, Summary of Investigations
    2000, Vol. 2, Saskatchewan Geological Survey, Sask. Energy Mines,
    Misc. Rep. 2000-4.2, in press.
  2. Interactions of Plutonium(V) and Plutonium(VI) with Manganese
    Dioxide, D. M. Smith, M. A. Ginder-Vogel, S. Skanthakumar,
    L. Soderholm, and M. P. Neu, Environmental Science and Technology,
    submitted
  3. Electronic and Magnetic Properties of Cm inPb2Sr2Cm1-xCaxCu3O8
    S. Skanthakumar, C. W. Williams and L. Soderholm, Phys. Rev. B.,
    submitted

 

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